Abstract
AbstractAerosol deposition is one of the major processes providing bioavailable Fe to the surface ocean. However, the quantification of aerosol Fe flux in the surface ocean is highly challenging operationally. In this study, we measured both Fe isotopic composition and specific elemental ratios in 5 size‐fraction aerosols collected over the East China Sea (ECS) to quantify the relative contribution of lithogenic and anthropogenic aerosol Fe. Both the isotopic and elemental ratios indicate that anthropogenic aerosol Fe mainly originates from high‐temperature combustion activities with the end member of the δ56Fe to be −4.5‰. We found that the Cd/Ti ratio is a much more reliable proxy to quantify the contribution of anthropogenic aerosol Fe in coarse aerosols than δ56Fe in the ECS. Attributed to extremely high deposition velocities and high total Fe concentrations for large size aerosols, lithogenic aerosols are still the dominant dissolved aerosol Fe source in the ECS.
Published Version
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.